This study
investigates the magnetic properties and critical current density of
Tl?Ba?Ca?Cu?O???? (Tl-2234)
high-temperature superconductors through AC magnetic susceptibility
measurements. Samples were synthesized using a one-step solid-state process
with careful heat treatment protocols to minimize thallium evaporation. AC
susceptibility measurements were conducted across temperatures ranging from 140
to 50K under various applied AC magnetic fields (0.5-8 mT). The analysis
revealed a sharp transition primarily reflecting intragranular
superconductivity, with the field dependence of the imaginary (?'') component
providing insights into flux dynamics within the grains. The imaginary
component peaks shifted towards lower temperatures with increasing magnetic
field strength, indicating enhanced magnetic field penetration and increased
intra-grain pinning centers. Using Bean's critical-state model, with an
estimated effective particle radius of R ? 44.5 µm based on sieve size, the
critical current density (Jc) was calculated from the peak positions
in ?''(T) curves. The temperature dependence of Jc followed an
empirical scaling relation, yielding a zero-temperature critical current
density Jc(0) of 3.6×10? A/cm² and a critical exponent of 1.26 ±
0.08, quantifying key superconducting parameters of the prepared material.